US2022227663A1PendingUtilityA1

Lithium Silicate-Low Quartz Glass Ceramic

Assignee: IVOCLAR VIVADENT AGPriority: Aug 25, 2015Filed: Apr 6, 2022Published: Jul 21, 2022
Est. expiryAug 25, 2035(~9.1 yrs left)· nominal 20-yr term from priority
C03C 10/0045C03B 19/066A61C 13/0006A61C 13/0004C03C 10/0027C03C 3/097C03C 4/0021A61K 6/833C03C 3/087C03C 2203/10
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Claims

Abstract

Lithium silicate-low quartz glass ceramics are described which are characterized by a combination of very good mechanical and optical properties and can therefore be used in particular as restoration material in dentistry.

Claims

exact text as granted — not AI-modified
1 . Lithium silicate-low quartz glass ceramic, which comprises lithium silicate as main crystal phase and low quartz as further crystal phase. 
     
     
         2 . Glass ceramic according to  claim 1 , which comprises 59.0 to 79.0 wt.-% SiO 2 . 
     
     
         3 . Glass ceramic according to  claim 1 , which comprises 8.0 to 15.0 wt.-% Li 2 O. 
     
     
         4 . Glass ceramic according to  claim 1 , which comprises 0 to 9.0 wt.-% P 2 O 5 . 
     
     
         5 . Glass ceramic according to  claim 1 , which comprises 1.0 to 8.0 wt.-% oxide of monovalent elements Me I   2 O selected from the group of K 2 O, Na 2 O, Rb 2 O, Cs 2 O and mixtures thereof. 
     
     
         6 . Glass ceramic according to  claim 1 , which comprises 1.0 to 9.0 wt.-% oxide of divalent elements Me II O selected from the group of CaO, MgO, SrO, ZnO and mixtures thereof. 
     
     
         7 . Glass ceramic according to  claim 1 , which comprises 1.0 to 6.0 wt.-% MgO. 
     
     
         8 . Glass ceramic according to  claim 1 , which comprises 0 to 8.0 wt.-% oxide of trivalent elements Me III   2 O 3  selected from the group of Al 2 O 3 , B 2 O 3 , Y 2 O 3 , La 2 O 3 , Ga 2 O 3 , In 2 O 3  and mixtures thereof. 
     
     
         9 . Glass ceramic according to  claim 1 , which comprises 1.0 to 6.0 wt.-% Al 2 O 3 . 
     
     
         10 . Glass ceramic according to  claim 1 , which comprises at least one of the following components in the amounts specified: 
       
         
           
                 
                 
                 
               
                     
                     
                 
                     
                   Component 
                   wt.-% 
                 
                     
                     
                 
                     
                   SiO 2   
                   59.0 to 79.0 
                 
                     
                   Li 2 O 
                   8.0 to 15.0 
                 
                     
                   P 2 O 5   
                   0 to 9.0 
                 
                     
                   MeI 2 O 
                   1.0 to 8.0 
                 
                     
                   MeIIO 
                   1.0 to 9.0 
                 
                     
                   MeIII 2 O 3   
                   0 to 8.0 
                 
                     
                   MeIVO 2   
                   0 to 10.0 
                 
                     
                   MeV 2 O 5   
                   0 to 8.0 
                 
                     
                   MeVIO 3   
                   0 to 5.0 
                 
                     
                   fluorine 
                   0 to 1.0, 
                 
                     
                     
                 
             
                
                
                
               
               
                
                
                
                
                
                
                
                
                
                
                
               
            
           
         
         wherein 
         Me I   2 O is selected from the group of K 2 O, Na 2 O, Rb 2 O, Cs 2 O and mixtures thereof, 
         Me II O is selected from the group of CaO, MgO, SrO, ZnO and mixtures thereof, 
         Me III   2 O 3  is selected from the group of Al 2 O 3 , B 2 O 3 , Y 2 O 3 , La 2 O 3 , Ga 2 O 3 , In 2 O 3  and mixtures thereof, 
         Me IV O 2  is selected from the group of ZrO 2 , TiO 2 , SnO 2 , CeO 2 , GeO 2  and mixtures thereof, 
         Me V   2 O 5  is selected from the group of V 2 O 5 , Ta 2 O 5 , Nb 2 O 5  and mixtures thereof, and 
         Me VI O 3  is selected from the group of WO 3 , MoO 3  and mixtures thereof. 
       
     
     
         11 . Glass ceramic according to  claim 1 , which comprises at least one of the following components in the amounts specified: 
       
         
           
                 
                 
                 
               
                     
                     
                 
                     
                   Component 
                   wt.-% 
                 
                     
                     
                 
                     
                   SiO 2   
                   59.0 to 79.0 
                 
                     
                   Li 2 O 
                   8.0 to 15.0 
                 
                     
                   P 2 O 5   
                   0 to 9.0 
                 
                     
                   K 2 O 
                   0 to 5.0 
                 
                     
                   Na 2 O 
                   0 to 2.0 
                 
                     
                   Rb 2 O 
                   0 to 8.0 
                 
                     
                   Cs 2 O 
                   0 to 7.0 
                 
                     
                   CaO 
                   0 to 3.0 
                 
                     
                   MgO 
                   0 to 6.0 
                 
                     
                   SrO 
                   0 to 4.0 
                 
                     
                   ZnO 
                   0 to 9.0 
                 
                     
                   Al 2 O 3   
                   1.0 to 6.0 
                 
                     
                   B 2 O 3   
                   0 to 4.0 
                 
                     
                   Y 2 O 3   
                   0 to 5.0 
                 
                     
                   La 2 O 3   
                   0 to 5.0 
                 
                     
                   Ga 2 O 3   
                   0 to 3.0 
                 
                     
                   In 2 O 3   
                   0 to 5.0 
                 
                     
                   ZrO 2   
                   0 to 3.0 
                 
                     
                   TiO 2   
                   0 to 4.0 
                 
                     
                   SnO 2   
                   0 to 3.0 
                 
                     
                   GeO 2   
                   0 to 9.0 
                 
                     
                   CeO 2   
                   0 to 4.0 
                 
                     
                   V 2 O 5   
                   0 to 2.0 
                 
                     
                   Ta 2 O 5   
                   0 to 5.0 
                 
                     
                   Nb 2 O 5   
                   0 to 5.0 
                 
                     
                   WO 3   
                   0 to 3.0 
                 
                     
                   MoO 3   
                   0 to 3.0 
                 
                     
                   fluorine 
                   0 to 1.0. 
                 
                     
                     
                 
             
                
                
                
               
               
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
               
            
           
         
       
     
     
         12 . Glass ceramic according to  claim 1 , which comprises SiO 2  and Li 2 O in a molar ratio in the range of from 2.2 to 4.1. 
     
     
         13 . Glass ceramic according to  claim 1 , which comprises lithium disilicate or lithium metasilicate as main crystal phase. 
     
     
         14 . Glass ceramic according to  claim 1 , which has at least 20 wt.-% lithium disilicate crystals. 
     
     
         15 . Glass ceramic according to  claim 1 , which has 0.2 to 28 wt.-% low quartz crystals. 
     
     
         16 . Glass ceramic comprising lithium silicate as main crystal phase and low quartz as further crystal phase or starting glass comprising nuclei for the crystallization of lithium metasilicate, lithium disilicate and/or low quartz, wherein the glass ceramic and the starting glass are present in the form of a powder, a granulate, a blank or a dental restoration. 
     
     
         17 . Process for the preparation of the glass ceramic according to  claim 1 , in which a starting glass is subjected to at least one heat treatment in the range of 700 to 900° C. 
     
     
         18 . Process according to  claim 17 , in which
 (a) the starting glass is subjected to a heat treatment at a temperature of 400 to 600° C. in order to form a starting glass with nuclei for the crystallization of lithium metasilicate, lithium disilicate and/or low quartz, and   (b) the starting glass with nuclei is subjected to a heat treatment at a temperature of 700 to 900° C. in order to form the lithium silicate-low quartz glass ceramic.   
     
     
         19 . Process of using the glass ceramic according to  claim 1  as dental material, for coating dental restorations or for the preparation of dental restorations. 
     
     
         20 . Process for the preparation of a dental restoration comprising a bridge, inlay, onlay, veneer, abutment, partial crown, crown or facet, in which the glass ceramic according to  claim 1  is given the shape of the desired dental restoration by pressing or machining.

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