US2021188836A1PendingUtilityA1

6-AMINOPYRIDIN-3-YL THIAZOLES AS MODULATORS OF RORyT

Assignee: JANSSEN PHARMACEUTICA NVPriority: Apr 27, 2016Filed: Feb 23, 2021Published: Jun 24, 2021
Est. expiryApr 27, 2036(~9.7 yrs left)· nominal 20-yr term from priority
C07D 417/14C07D 417/04C07D 491/107C07D 487/08A61P 1/04A61P 3/00A61P 19/02C07D 491/08C07D 498/08C07B 59/002C07B 2200/05A61P 25/00A61K 31/4439A61P 37/00A61P 11/00A61P 29/00A61P 11/06A61P 37/02A61P 17/06A61P 43/00A61P 25/24
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Claims

Abstract

The present invention comprises compounds of Formula I.wherein:A1, A2, A3, A4, A5, R1, and R2 are defined in the specification.The invention also comprises a method of treating or ameliorating a syndrome, disorder or disease, wherein the syndrome, disorder or disease is rheumatoid arthritis or psoriasis. The invention also comprises a method of modulating RORγt activity in a mammal by administration of a therapeutically effective amount of at least one compound of Formula I.

Claims

exact text as granted — not AI-modified
We claim: 
     
         1 . A compound of Formula I. 
       
         
           
           
               
               
           
         
       
       wherein
 R 1  is H, —C (1-3) alkyl, —CHF 2 , —CF 3 , —CN, —OCH 3 , —OCH2CH 3 , cyclopropyl, OCF 3 , or OCHF 2 ; 
 R 2  is H, F, —CHF 2 , —CF 3 , —CN, —OCH 3 , —OCHF 2 , or OCF3; provided that R 2  may not be H if 1e is H; 
 A l  and A 2  are taken together with their attached nitrogen to form a ring selected from the group consisting of 
 
       
         
           
           
               
               
           
         
       
       or A 3  may be —CH 2 C(CH 3 ) 2 OH, when A 1  and A 2  are 
       
         
           
           
               
               
           
         
       
       A 4  is —H, or —CH 3 ;
 or A 3  and A 4  may be taken together with their attached nitrogen to form a ring selected from the group consisting of 
 
       
         
           
           
               
               
           
         
         A 5  is 
       
       
         
           
           
               
               
           
         
       
       wherein said —C (1-6) alkyl and —C (4-6) cycloalkyl are optionally substituted with up to three fluorine atoms; and said —C (1-6) alkyl is independently optionally substituted with one cyclobutyl, or up to two cyclopropyl groups;
 and pharmaceutically acceptable salts thereof. 
 
     
     
         2 . The compound of  claim 1  wherein:
 A 5  is 
 
       
         
           
           
               
               
           
         
       
       wherein said —C (3-6) alkyl and —C (4-6) cycloalkyl are optionally substituted with up to three fluorine atoms;
 and pharmaceutically acceptable salts thereof. 
 
     
     
         3 . The compound of  claim 2  wherein:
 R 1  is H, —C (1-3) alkyl, —CHF 2 , —CF 3 , —CN, —OCH 3 , —OCH 2 CH 3 , or cyclopropyl; 
 R 2  is H, F, —CHF 2 , —CF 3 , —CN, —OCH 3 , or —OCHF2; provided that R 2  may not be H if R 1  is H; 
 
       and pharmaceutically acceptable salts thereof. 
     
     
         4 . The compound of  claim 3  wherein:
 A 3  and A 4  may be taken together with their attached nitrogen to form a ring selected from the group consisting of 
 
       
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts thereof. 
     
     
         5 . The compound of  claim 4  wherein:
 A 1  and A 2  are taken together with their attached nitrogen to form a ring selected from the group consisting of 
 
       
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts thereof. 
     
     
         6 . The compound of  claim 3  selected from the group consisting of: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts thereof. 
     
     
         7 . The compound of  claim 3  selected from the group consisting of: 
       
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts thereof. 
     
     
         8 . The compound of  claim 4  selected from the group consisting of: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts thereof. 
     
     
         9 . The compound of  claim 5  selected from the group consisting of: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts thereof. 
     
     
         10 . A pharmaceutical composition, comprising a compound of  claim 1  and a pharmaceutically acceptable carrier. 
     
     
         11 . A method for treating or ameliorating a RORγt mediated inflammatory syndrome, disorder or disease selected from the group consisting of: inflammatory bowel diseases, rheumatoid arthritis, psoriasis, chronic obstructive pulmonary disorder, psoriatic arthritis, ankylosing spondylitis, neutrophilic asthma, steroid resistant asthma, multiple sclerosis, and systemic lupus erythematosus, comprising administering to a subject in need thereof an effective amount of a compound of  claim 1 . 
     
     
         12 . A method for treating or ameliorating a RORγt mediated inflammatory syndrome, disorder or disease selected from the group consisting of: depression and metabolic syndrome, comprising administering to a subject in need thereof an effective amount of a compound of  claim 1 . 
     
     
         13 . The method of  claim 11 , wherein the disease is psoriasis. 
     
     
         14 . The method of  claim 11 , wherein the disease is rheumatoid arthritis. 
     
     
         15 . The method of  claim 11 , wherein the inflammatory bowel disease is ulcerative colitis. 
     
     
         16 . The method of  claim 11 , wherein the inflammatory bowel disease is Crohn's disease. 
     
     
         17 . The method of  claim 11 , wherein the disease is multiple sclerosis. 
     
     
         18 . The method of  claim 11 , wherein the disease is neutrophilic asthma. 
     
     
         19 . The method of  claim 11 , wherein the disease is steroid resistant asthma. 
     
     
         20 . The method of  claim 11 , wherein the disease is psoriatic arthritis. 
     
     
         21 . The method of  claim 11 , wherein the disease is ankylosing spondylitis. 
     
     
         22 . The method of  claim 11 , wherein the disease is systemic lupus erythematosus. 
     
     
         23 . The method of  claim 11 , wherein the disease is chronic obstructive pulmonary disorder. 
     
     
         24 . The method of  claim 12 , wherein the disease is depression. 
     
     
         25 . The method of  claim 12 , wherein the disease is metabolic syndrome. 
     
     
         26 . A method of inhibiting production of interleukin-17, comprising administering to a subject in need thereof an effective amount of a compound of  claim 1 .

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