US2018296345A1PendingUtilityA1

Substrate with a Structured Surface and Methods for the Production Thereof, and Methods for Determining the Wetting Properties Thereof

Assignee: JENNISSEN HERBERTPriority: Dec 16, 2011Filed: Jun 20, 2018Published: Oct 18, 2018
Est. expiryDec 16, 2031(~5.4 yrs left)· nominal 20-yr term from priority
C23C 4/18A61L 27/04G01N 2013/0291C23C 4/08A61L 2400/18A61L 27/50C23C 4/134A61F 2/28G01N 13/02A61L 17/145A61F 2002/2835G01N 2013/0283A61F 2310/00011B23K 26/0066B23K 26/352
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Claims

Abstract

An implant includes a microstructured hyperhydrophilic surface with protrusions and depressions in which a spacing between the protrusions as a statistical mean is in a range of 1 to 100 μm and a profile height of the protrusions and depressions as a statistical mean is in the range of 1 to 80 μm.

Claims

exact text as granted — not AI-modified
1 . A method for the production of an implant with a regularly microstructured surface with protrusions and depressions, wherein the spacing between the protrusions as the statistical mean is in a range of 1 to 100 μm and a profile height of the protrusions and depressions as a statistical mean is in a range of 1 to 80 μm, and wherein the implant has a microscopic roughness factor r M  in a range between 2 and 50, comprising:
 a) providing a powder or a powder mixture of a sinterable material powder on a blank; 
 b) applying a layer of the metal powder to the surface of the blank; and 
 c) acting on the layer of the material powder with energy-rich radiation in a pattern which can be represented from a periodic function converted into an STL data set so that material powder is sintered on at least a partial region of the surface of the blank with the formation of at least a partial region of the pattern. 
 
     
     
         2 . A method according to  claim 1  wherein the blank is produced from solid material or layer-wise by way of a sintering method from a sinterable material powder. 
     
     
         3 . A method according to  claim 1  wherein the blank obtained in c) with a regularly microstructured surface is subjected to a treatment for producing a second regular microstructure using a periodic function converted into an STL data set and/or a wet-chemical treatment for producing a nanostructure. 
     
     
         4 . A method for the production of an implant with a regularly microstructured surface, comprising:
 a) providing a blank; and   b) acting on the blank with energy-rich radiation at least partially in a pattern which can be represented from a periodic function converted into an STL data set so that the blank is ablated with the formation of at least a partial region of the pattern on at least a partial region of the surface.   
     
     
         5 . A method according to  claim 4  in which the blank obtained in b) with a regularly microstructured surface is subjected to a treatment for producing a second regular microstructure using a periodic function converted into an STL data set and/or a wet-chemical treatment for producing a nanostructure. 
     
     
         6 . A method according to  claim 3  wherein the treatment for producing a nanostructure includes the step of a wet-chemical treatment of the microstructured surface,
 wherein a hydrophobic or weakly hydrophilic surface is converted to an ultrahydrophilic or hyperhydrophilic surface, wherein at least one of the two dynamic contact angles θ V  and θ R  is in the hyperhydrophilic range with 1.0<ΔF/P·γ≤2.15, wherein θ ai >0.0i°−80i°, 
 wherein θ V  stands for advancing angle, θ R  stands for receding angle, ΔF stands for a difference between measured net forces, γ stands for surface tension of water, and P stands for perimeter of the sample. 
 
     
     
         7 . A method according to  claim 6  which further comprises the additional step that the surface obtained is protected, stabilised and rendered capable of long-term storage by a solution of non-volatile substances like salts, organic solvents which do not interact with the surface, or a salt-bearing exsiccation layer for protecting the surface of the substrate in relation to a reduction in wetting with a loss of hyperhydrophilia due to aging or stabilisation methods. 
     
     
         8 . A method according to  claim 1  in which the periodic function converted into an STL data set is a trigonometric function A R (x) selected from the group consisting of: 
       
         
           
             
               
                 
                   
                     
                         
                     
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       and derivatives thereof. 
     
     
         9 . A method according to  claim 1  in which the roughness parameter is in the range of between 1 and 80 μm. 
     
     
         10 . A method according to  claim 1  in which a periodicity value n(λ/2) is in the range of between 1 and 100 μm. 
     
     
         11 . A method for determining the wetting properties of the surface of a substrate, comprising:
 a) carrying out a Wilhelmy/force measurement for ascertaining (K θ ·F),   b) calculating the apparent contact angles θ V  and θ R  on the basis of the result of step a), wherein said calculation
 i. is effected for the situation where (K θ ·F)≤1 in accordance with arccos (K θ ·F)=real contact angles; and 
 ii. is effected for the situation where (K θ ·F)>1 in accordance with arccos(K θ ·F)=imaginary contact angles; and 
   c) determining the wetting properties of the substrate on the basis of the contact angles θ V  and θ R  calculated in step b).   
     
     
         12 . An apparatus for carrying out the method according to  claim 11  comprising:
 a measuring unit, an evaluation unit and an output unit, 
 wherein the measuring unit is adapted for force measurement of the Wilhelmy/force measurement, 
 wherein the evaluation unit is adapted to convert the measurement values obtained by the measuring unit by an algorithm into an imaginary advancing angle (θ V ) and receding angle (θ R ) and 
 wherein the output unit is adapted to further process the contact angle obtained by the evaluation unit. 
 
     
     
         13 . The method according to  claim 3 , wherein at least one of two dynamic contact angles θ V  and θ R  is in a hyperhydrophilic range with 1.0<ΔF/P·γ≤1.0619, wherein θ ai >0.0i°−20i°,
 wherein θ V  stands for advancing angle, θ R  stands for receding angle, ΔF stands for a difference between measured net forces, γ stands for surface tension of water, and P stands for perimeter of the sample.

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