US2018079774A1PendingUtilityA1

Substituted nucleosides, nucleotides and analogs thereof

Assignee: ALIOS BIOPHARMA INCPriority: Jun 26, 2013Filed: Oct 27, 2017Published: Mar 22, 2018
Est. expiryJun 26, 2033(~6.9 yrs left)· nominal 20-yr term from priority
A61P 31/14A61P 31/12C07H 19/20C07H 19/16C07H 19/06C07H 19/10C07H 19/11
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Claims

Abstract

Disclosed herein are nucleosides, nucleotides and analogs thereof, pharmaceutical compositions that include one or more of nucleosides, nucleotides and analogs thereof, and methods of synthesizing the same. Also disclosed herein are methods of ameliorating and/or treating a disease and/or a condition, including an infection from a norovirus, with a nucleoside, a nucleotide and an analog thereof.

Claims

exact text as granted — not AI-modified
1 . A method for ameliorating, treating or preventing a norovirus infection comprising contacting a cell infected with the norovirus with an effective amount of a compound of Formula (II) or Formula (III), or a pharmaceutically acceptable salt of the foregoing, wherein Formula (II) and Formula (III) are: 
       
         
           
           
               
               
           
         
         wherein: 
         B 1B  and B 1C  are independently an optionally substituted heterocyclic base or an optionally substituted heterocyclic base with a protected amino group; 
         R 1B  is selected from the group consisting of O − , OH, an optionally substituted C 1-6  alkoxy, 
       
       
         
           
           
               
               
           
         
       
       an optionally substituted N-linked amino acid and an optionally substituted N-linked amino acid ester derivative;
 R 1C  and R 2C  are independently selected from the group consisting of O − , OH, an optionally substituted C 1-6  alkoxy, 
 
       
         
           
           
               
               
           
         
       
       an optionally substituted N-linked amino acid and an optionally substituted N-linked amino acid ester derivative; or
 R 1C  is 
 
       
         
           
           
               
               
           
         
       
       and R 2C  is O −  or OH;
 R 2B  and R 3C  are independently selected from the group consisting of halogen, an optionally substituted C 1-6  alkyl, an optionally substituted C 2-6  alkenyl, an optionally substituted C 2-6  alkynyl, an optionally substituted C 3-6  cycloalkyl, an optionally substituted —O—C 1-6  alkyl, an optionally substituted —O—C 3-6  alkenyl, an optionally substituted —O—C 3-6  alkynyl and cyano; 
 R 4C  is selected from the group consisting of OH, —OC(═O)R″ C  and an optionally substituted O-linked amino acid; 
 R 3B  and R 5C  are independently selected from the group consisting of hydrogen, halogen, OR 1D , an optionally substituted O-linked amino acid, azido and NR 2D R 3D ; 
 R 1D  is hydrogen or —C(═O)R″ D ; 
 R 2D  and R 3D  are independently hydrogen or an optionally substituted C 1-6  alkyl; 
 R 4B  and R 6C  are independently selected from the group consisting of hydrogen, halogen, an optionally substituted C 1-6  alkyl, an optionally substituted C 2-6  alkenyl and an optionally substituted C 2-6  alkynyl; 
 R 5B , R 6B , R 8B , R 9B , R 9C , R 10C , R 12C  and R 13C  are independently selected from the group consisting of hydrogen, an optionally substituted C 1-24  alkyl and an optionally substituted aryl; 
 R 7B , R 10B , R 11C  and R 14C  are independently selected from the group consisting of hydrogen, an optionally substituted C 1-24  alkyl, an optionally substituted aryl, an optionally substituted —O—C 1-24  alkyl, an optionally substituted —O-aryl, an optionally substituted —O-heteroaryl, an optionally substituted —O-monocyclic heterocyclyl and 
 
       
         
           
           
               
               
           
         
         R 11B1 , R 11B2 , R 15C1  and R 15C2  are independently selected from the group consisting of hydrogen, an optionally substituted C 1-24  alkyl and an optionally substituted aryl; 
         R 16C , R 17C  and R 18C  are independently absent or hydrogen; 
         for Formula (III),   is a single bond or a double bond;
 when   is a single bond, each R 7C  and each R 8C  is independently hydrogen or halogen; and 
 when   is a double bond, each R 7C  is absent and each R 8C  is independently hydrogen or halogen; 
 
         R″ C  and R″ D  are independently an optionally substituted C 1-24 -alkyl; 
         d and j are independently 1 or 2; 
         e1 and k1 are independently 0 or 1; 
         e2 and k2 are independently 3, 4 or 5; 
         n is 0 or 1; 
         Z 1B , Z 2B  and Z 1C  are independently O or S. 
       
     
     
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         115 . The method of  claim 1 , wherein the compound is a compound of Formula (II). 
     
     
         116 . The method of  claim 115 , wherein R 1B  is O −  or OH. 
     
     
         117 . The method of  claim 115 , wherein R 1B  is an optionally substituted C 1-6  alkoxy, 
       
         
           
           
               
               
           
         
       
     
     
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         122 . The method of  claim 115 , wherein R 1B  is an optionally substituted N-linked amino acid or an optionally substituted N-linked amino acid ester derivative. 
     
     
         123 . The method of  claim 115 , wherein R 1B  is selected from the group consisting of alanine, asparagine, aspartate, cysteine, glutamate, glutamine, glycine, proline, serine, tyrosine, arginine, histidine, isoleucine, leucine, lysine, methionine, phenylalanine, threonine, tryptophan, valine and ester derivatives thereof. 
     
     
         124 . The method of  claim 115 , wherein R 1B  is selected from the group consisting of alanine isopropyl ester, alanine cyclohexyl ester, alanine neopentyl ester, valine isopropyl ester and leucine isopropyl ester. 
     
     
         125 . The method of  claim 115 , wherein R 1B  has the structure 
       
         
           
           
               
               
           
         
       
       wherein R 12B  is selected from the group consisting of hydrogen, an optionally substituted C 1-6 -alkyl, an optionally substituted C 3-6  cycloalkyl, an optionally substituted aryl, an optionally substituted aryl(C 1-6  alkyl) and an optionally substituted haloalkyl; R 13B  is selected from the group consisting of hydrogen, an optionally substituted C 1-6  alkyl, an optionally substituted C 1-6  haloalkyl, an optionally substituted C 3-6  cycloalkyl, an optionally substituted C 6  aryl, an optionally substituted C 10  aryl and an optionally substituted aryl(C 1-6  alkyl); and R 14B  is hydrogen or an optionally substituted C 1-4 -alkyl; or R 13B  and R 14B  are taken together to form an optionally substituted C 3-6  cycloalkyl. 
     
     
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         138 . The method of  claim 115 , wherein R 2B  is unsubstituted C 1-6  alkyl, unsubstituted C 2-6  alkenyl, unsubstituted C 2-6  alkynyl, unsubstituted —O—C 1-6  alkyl, unsubstituted —O—C 3-6  alkenyl or unsubstituted —O—C 3-6  alkynyl. 
     
     
         139 . The method of  claim 115 , wherein R 2B  is cyano. 
     
     
         140 . The method of  claim 115 , wherein R 4B  is hydrogen. 
     
     
         141 . The method of  claim 115 , wherein R 4B  is halogen. 
     
     
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         146 . The method of  claim 115 , wherein R 3B  is hydrogen, halogen, OR 1D , OH, or —OC(═O)R″ D . 
     
     
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         152 . The method of  claim 115 , wherein R 3B  is an optionally substituted O-linked amino acid, azido, NR 2D R 3D , or NH 2 . 
     
     
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         158 . The method of  claim 115 , wherein Z 1B  is O. 
     
     
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         160 . The method of  claim 115 , wherein B 1B  is selected from the group consisting of: 
       
         
           
           
               
               
           
         
         wherein: 
         R AB2  is selected from the group consisting of hydrogen, halogen and NHR JB2 , wherein R JB2  is selected from the group consisting of hydrogen, —C(═O)R KB2  and —C(═O)OR LB2 ; 
         R BB2  is halogen or NHR WB2 , wherein R WB2  is selected from the group consisting of hydrogen, an optionally substituted C 1-6  alkyl, an optionally substituted C 2-6  alkenyl, an optionally substituted C 3-8  cycloalkyl, —C(═O)R MB2  and —C(═O)OR NB2 ; 
         R CB2  is hydrogen or NHR OB2 , wherein R OB2  is selected from the group consisting of hydrogen, —C(═O)R PB2  and —C(═O)OR QB2 ; 
         R DB2  is selected from the group consisting of hydrogen, deuterium, halogen, an optionally substituted C 1-6  alkyl, an optionally substituted C 2-6  alkenyl and an optionally substituted C 2-6  alkynyl; 
         R EB2  is selected from the group consisting of hydrogen, hydroxy, an optionally substituted C 1-6  alkyl, an optionally substituted C 3-8  cycloalkyl, —C(═O)R RB2  and —C(═O)OR SB2 ; 
         R FB2  is selected from the group consisting of hydrogen, halogen, an optionally substituted C 1-6 alkyl, an optionally substituted C 2-6  alkenyl and an optionally substituted C 2-6  alkynyl; 
         Y 2B  and Y 3B  are independently N or CR IB2 , wherein R B2  is selected from the group consisting of hydrogen, halogen, an optionally substituted C 1-6 -alkyl, an optionally substituted C 2-6 -alkenyl and an optionally substituted C 2-6 -alkynyl; 
         R GB2  is an optionally substituted C 1-6  alkyl; 
         R HB2  is hydrogen or NHR TB2 , wherein R TB2  is independently selected from the group consisting of hydrogen, —C(═O)R UB2  and —C(═O)OR VB2 ; and 
         R KB2 , R LB2 , R MB2 , R NB2 , R PB2 , R QB2  R RB2 , R SB2 , R UB2  and R VB2  are independently selected from the group consisting of C 1-6  alkyl, C 2-6  alkenyl, C 2-6  alkynyl, C 3-6  cycloalkyl, C 3-6  cycloalkenyl, C 6-10  aryl, heteroaryl, heteroalicyclyl, aryl(C 1-6  alkyl), heteroaryl(C 1-6  alkyl) and heteroalicyclyl(C 1-6  alkyl). 
       
     
     
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         167 . The method of  claim 1 , wherein the compound is a compound of Formula (III). 
     
     
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         236 . The method of  claim 115 , wherein the compound of Formula (II) is selected from the group consisting of: 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable salt thereof. 
     
     
         237 . The method of  claim 115 , wherein the compound of Formula (II) is selected from the group consisting of: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable salt of the foregoing. 
     
     
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