US2017002178A1PendingUtilityA1

Stabilizer mixture

Assignee: BASF SEPriority: Jan 13, 2006Filed: Sep 19, 2016Published: Jan 5, 2017
Est. expiryJan 13, 2026(expired)· nominal 20-yr term from priority
C08K 5/3435C08L 2201/08C08L 23/12C07B 63/04C09K 15/30C09D 7/65C09D 7/48C08K 2201/014C07D 211/58C08K 5/34C09K 15/20
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Claims

Abstract

Suitable stabilizers for organic material are a mixture comprising A. at least one oligomeric compound, comprising repeat units of the formula (I), in which the meanings of the symbols are as follows: R1 is hydrogen, C1-C6-alkyl, formyl, C2-C6-alkanoyl, C1-C12-alkoxy, C5-C6-cycloalkoxy, cyanomethyl, 2-hydroxyethyl, benzyl or a radical of the formula -CR'=CH-CO-OR'', where R' is hydrogen, C1-C6-alkyl or a radical of the formula -CO-OR'', and R'' is C1-C18-alkyl, C5-C8-cycloalkyl, C7-C18-aralkyl, phenyl, or tolyl; R2 is a mixture composed of C14-C25-alkyl groups, where two of these alkyl groups whose number of carbon atoms is not permitted to differ by more than two respectively make up at least 30% of this mixture; R3 and R4, independently of one another, are C1-C6-alkyl; and B. at least one compound of the formula (II) or (III) where the meanings of the symbols and indices are as follows: n and m, independently of one another, are a natural number from 2 to 22, and R1, R3 and R4, independently of one another, have the meanings given in formula (I).

Claims

exact text as granted — not AI-modified
1 . A mixture, comprising
 (A) at least one oligomeric compound, comprising repeat units of the formula (I),   
       
         
           
           
               
               
           
         
         wherein: 
         R 1  is hydrogen, C 1 -C 6 -alkyl, formyl, C 2 -C 6 -alkanoyl, C 1 -C 12 -alkoxy, C 5 -C 6 -cycloalkoxy, cyanomethyl, 2-hydroxyethyl, benzyl or a radical of the formula —CR′═CH—CO—OR″, wherein
 R′ is hydrogen, C 1 -C 6 -alkyl or a radical of the formula —CO—OR″, and 
 R″ is C 1 -C 18 -alkyl, C 5 -C 8 -cycloalkyl, C 7 -C 18 -aralkyl, phenyl, or tolyl; 
 
         R 2  is a mixture composed of C 14 -C 28 -alkyl groups, where two of these alkyl groups whose number of carbon atoms is not permitted to differ by more than two respectively make up at least 30% of this mixture; 
         R 3  and R 4 , independently of one another, are C 1 -C 6 -alkyl; 
         and 
         (B) at least one compound of the formula (II) or (III) 
       
       
         
           
           
               
               
           
         
         wherein: 
         n and m, independently of one another, are a natural number from 2 to 22, 
         and 
         R 1 , R 3  and R 4 , independently of one another, have the meanings given are as defined in formula (I). 
       
     
     
         2 . The mixture according to  claim 1 ,
 wherein:   R 1  is H, C 1 -C 6 -alkyl, formyl, acyl, or benzyl;   R 2  is a mixture composed of C 16 -C 24 -alkyl groups;   R 3  and R 4  are methyl; and   m and n are a natural number from 6 to 8.   
     
     
         3 . The mixture according to  claim 1 , wherein component A is an oligomer of formula (Ia): 
       
         
           
           
               
               
           
         
         and component B has been selected from the group of the compounds (IIa), (IIIa), and (IIIb): 
       
       
         
           
           
               
               
           
         
       
     
     
         4 . A process for preparation of a mixture according to  claim 1 , comprising:
 a) adding component (B) to a melt of component (A) to obtain a mixture;   b) homogenizing the mixture to obtain a resultant mixture; and   c) converting the resultant mixture to a desired form and allowing to cool.   
     
     
         5 . An organic material stabilized with respect to exposure to light, oxygen, and heat, comprising from 0.01 to 5% by weight, based on the amount of the organic material, of a mixture according to  claim 1 . 
     
     
         6 . A plastic or paint stabilized with respect to exposure to light, oxygen, and heat, comprising from 0.01 to 5% by weight, based on the amount of the organic material, of a mixture according to  claim 1 . 
     
     
         7 . The mixture according to  claim 1 , wherein the mixture is suitable as light stabilizers and other stabilizers for organic material. 
     
     
         8 . The mixture according to  claim 7 , wherein the mixture is suitable as light stabilizers and other stabilizers for plastics and paints. 
     
     
         9 . A method for stabilization of organic material with respect to exposure to light, oxygen, and heat, adding a mixture according to  claim 1  to the organic material. 
     
     
         10 . A method for stabilization of plastics and paints with respect to exposure to light, oxygen, and heat, adding a mixture according to  claim 1  to the plastics, paint, or a combination thereof. 
     
     
         11 . A tape, comprising:
 a polypropylene; and   a mixture, comprising
 (A) at least one oligomeric compound, comprising repeat units of the formula (I), 
   
       
         
           
           
               
               
           
         
         
           wherein: 
           R 1  is hydrogen, C 1 -C 6 -alkyl, formyl, C 2 -C 6 -alkanoyl, C 1 -C 12 -alkoxy, C 5 -C 6 -cycloalkoxy, cyanomethyl, 2-hydroxyethyl, benzyl or a radical of the formula —CR′═CH—CO—OR″, wherein
 R′ is hydrogen, C 1 -C 6 -alkyl or a radical of the formula —CO—OR″, and 
 R″ is C 1 -C 18 -alkyl, C 5 -C 8 -cycloalkyl, C 7 -C 18 -aralkyl, phenyl, or tolyl; 
 
           R 2  is a mixture composed of C 14 -C 28 -alkyl groups, where two of these alkyl groups whose number of carbon atoms is not permitted to differ by more than two respectively make up at least 30% of this mixture; 
           R 3  and R 4 , independently of one another, are C 1 -C 6 -alkyl; and 
           (B) at least one compound of the formula (II) or (III) 
         
       
       
         
           
           
               
               
           
         
         
           wherein: 
           n and m, independently of one another, are a natural number from 2 to 22, and 
           R 1 , R 3  and R 4 , independently of one another, are as defined in formula (I). 
         
       
     
     
         12 . The tape according to  claim 11 , wherein:
 R 1  is H, C 1 -C 6 -alkyl, formyl, acyl, or benzyl;   R 2  is a mixture composed of C 16 -C 24 -alkyl groups;   R 3  and R 4  are methyl; and   m and n are a natural number from 6 to 8.   
     
     
         13 . The tape according to  claim 11 , wherein component A is an oligomer of formula (Ia): 
       
         
           
           
               
               
           
         
         and component B has been selected from the group of the compounds (IIa), (IIIa), and (IIIb):

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