US2008182980A1PendingUtilityA1

Reactive Functional Groups

Assignee: THIRD WAVE TECH INCPriority: Jan 6, 2003Filed: Nov 20, 2007Published: Jul 31, 2008
Est. expiryJan 6, 2023(expired)· nominal 20-yr term from priority
C07H 21/04
58
PatentIndex Score
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Cited by
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Claims

Abstract

The present invention relates to compositions and methods for the preparation of modified nucleic acids. In particular, the present invention provides novel reagents and chemistries for the generation of linkers and modified phosphoramidates.

Claims

exact text as granted — not AI-modified
1 . A composition comprising: 
       
         
           
           
               
               
           
         
       
     
     
         2 . A modified CPG, said CPG comprising the composition of  claim 1 . 
     
     
         3 . A modified phosphoramidite comprising the composition of  claim 1 . 
     
     
         4 . A composition comprising a nucleic acid, said nucleic acid comprising the structure: 
       
         
           
           
               
               
           
         
       
     
     
         5 . A composition comprising a nucleic acid, said nucleic acid comprising the structure:
   (5′)HO-Nucleic Acid-O—P(O 2 )—O—(CH 2 ) 6 —CH 2 —NH—R.   
     
     
         6 . The composition of  claim 5 , wherein R is a label. 
     
     
         7 . The composition of  claim 6 , wherein said label is selected from the group consisting of fluorescent labels, chemiluminescent labels, and enzymatically reactive labels. 
     
     
         8 . The composition of  claim 5 , wherein R is a biological molecule. 
     
     
         9 . A composition comprising a phosphoramidite, said phosphoramidite comprising the structure 
       
         
           
           
               
               
           
         
       
     
     
         10 . The composition of  claim 9 , wherein R is selected from the group consisting of C 6 H 12  and polyethylene glycol 3400. 
     
     
         11 . The composition of  claim 9 , wherein R is a label. 
     
     
         12 . The composition of  claim 11 , wherein said label is selected from the group consisting of fluorescent labels, chemiluminescent labels, and enzymatically reactive labels. 
     
     
         13 . The composition of  claim 9 , wherein R is a biological molecule. 
     
     
         14 . A composition comprising the structure: 
       
         
           
           
               
               
           
         
       
     
     
         15 . The composition of  claim 14 , wherein R is a label. 
     
     
         16 . The composition of  claim 15 , wherein said label is selected from the group consisting of fluorescent labels, chemiluminescent labels, and enzymatically reactive labels. 
     
     
         17 . The composition of  claim 14 , wherein R is a biological molecule. 
     
     
         18 . A composition comprising a nucleic acid, said nucleic acid comprising a structure selected from the group consisting of:
   (3′)OH-nucleic acid-O—P(O 2 )—O—C 6 H 12 —NH—C(O)—(CH 2 ) 7 —CH(OH)—CH(OH)—(CH 2 ) 6 —O-DMT     and     (3′)OH-nucleic acid-O—P(O 2 )—O—C 6 H 12 —NH—(O)C—(CH 2 ) 7 —CH(OH)—CH(OH)—(CH 2 ) 6 —O—P(O 2 )—O—R—OH     and     (3′)OH-nucleic acid-O—P(O 2 )—O—C 6 H 12 —NH—(O)C—(CH 2 ) 7 —C(O)H     and     (3′)OH-nucleic acid O—P(O 2 )—O—C 6 H 12 —NH—(O)C—(CH 2 ) 7 —CH(OH)—CH(OH)—(CH 2 ) 6 —O—P(O 2 )—O-nucleic acid-O—P(O 2 )-FAM   
     
     
         19 . The composition of  claim 9 , wherein R is C 12 H 25 . 
     
     
         20 . A kit comprising a nucleic acid labeling reagent selected from the group consisting of:
                     (3′)OH-nucleic acid-O—P(O 2 )—O—C 6 H 12 —NH—C(O)—(CH 2 ) 7 —CH(OH)—CH(OH)—(CH 2 ) 6 —O-DMT     and     (3′)OH-nucleic acid-O—P(O 2 )—O—C 6 H 12 —NH—(O)C—(CH 2 ) 7 —CH(OH)—CH(OH)—(CH 2 ) 6 —O—P(O 2 )—O—R 3 —OH     and     (3′)OH-nucleic acid-O—P(O 2 )—O—C 6 H 12 —NH—(O)C—(CH 2 ) 7 —C(O)H     and (3′)OH-nucleic acid-O—P(O 2 )—O—C 6 H 12 —NH—(O)C—(CH 2 ) 7 —CH(OH)—CH(OH)—(CH 2 ) 6 —O—P(O 2 )—O-nucleic acid-O—P(O 2 )-FAM   
     
     
         21 . The kit of  claim 20 , wherein R 1  is selected from the group consisting of C 6 H 12  and polyethylene glycol 3400. 
     
     
         22 . The kit of  claim 20 , wherein R 1 , R 2  and R 3  are labels. 
     
     
         23 . The kit of  claim 22 , wherein said labels are selected from the group consisting of fluorescent labels, chemiluminescent labels, and enzymatically reactive labels. 
     
     
         24 . The kit of  claim 20 , wherein R 1 , R 2  and R 3  are biological molecules. 
     
     
         25 . The kit of  claim 9 , wherein R 3  is C 12 H 25 . 
     
     
         26 . A method of labeling nucleic acids, comprising
 a) providing a nucleic acid labeling reagent selected from the group consisting of
                     (3′)OH-nucleic acid-O—P(O 2 )—O—C 6 H 12 —NH—C(O)—(CH 2 ) 7 —CH(OH)—CH(OH)—(CH 2 ) 6 —O-DMT 
   and 
   (3′)OH-nucleic acid-O—P(O 2 )—O—C 6 H 12 —NH—(O)C—(CH 2 ) 7 —CH(OH)—CH(OH)—(CH 2 ) 6 —O—P(O 2 )—O—R 3 —OH 
   and 
   (3′)OH-nucleic acid-O—P(O 2 )—O—C 6 H 12 —NH—(O)C—(CH 2 ) 7 —C(O)H 
   and 
   nucleic acid-O—P(O 2 )—O—C 6 H 12 —NH—(O)C—(CH 2 ) 7 —CH(OH)—CH(OH)—(CH 2 ) 6 —O—P(O 2 )—O-nucleic acid-O—P(O 2 )-FAM; 
   
       and
 b) contacting said nucleic acid labeling reagent with a nucleic acid under conditions such that said nucleic acid labeling reagent is covalently linked to said nucleic acid. 
 
     
     
         27 . The method of  claim 26 , wherein said nucleic acid labeling reagent is attached to a CPG. 
     
     
         28 . The method of  claim 26 , wherein said nucleic acid labeling reagent is attached to a second nucleic acid. 
     
     
         29 . The method of  claim 26 , wherein said nucleic acid labeling reagent is attached to a solid support. 
     
     
         30 . The method of  claim 29 , wherein said solid support comprises an array of said nucleic acid labeling reagents. 
     
     
         31 . The method of  claim 26 , wherein said nucleic acid is an oligonucleotide. 
     
     
         32 . The method of  claim 26 , wherein R 1  is selected from the group consisting of C 6 H 12  and polyethylene glycol 3400. 
     
     
         33 . The method of  claim 26 , wherein R 1 , R 2  and R 3  are labels. 
     
     
         34 . The method of  claim 33 , wherein said labels are selected from the group consisting of fluorescent labels, chemiluminescent labels, and enzymatically reactive labels. 
     
     
         35 . The method of  claim 33 , wherein R 1 , R 2  and R 3  are biological molecules. 
     
     
         36 . The method of  claim 26 , wherein R 3  is C 12 H 25 .

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