US2008167310A1PendingUtilityA1

Modulators of peroxisome proliferator activated receptors (ppar)

Assignee: GOSSETT LYNN STACYPriority: Jun 7, 2001Filed: Oct 3, 2007Published: Jul 10, 2008
Est. expiryJun 7, 2021(expired)· nominal 20-yr term from priority
A61P 43/00A61P 9/12A61P 9/04A61P 9/00A61P 3/10A61P 9/10A61P 3/06C07D 277/28C07D 231/12C07C 233/63C07D 333/28C07D 417/14A61P 25/00C07D 413/14C07D 413/12C07D 417/04C07D 409/12C07D 413/04C07D 263/32C07C 2601/14C07D 213/81C07D 417/12C07D 277/42A61P 3/04C07C 233/87C07D 495/04A61P 3/02C07D 401/06C07D 209/48C07D 239/28C07D 413/06C07C 271/22C07C 271/24C07C 255/57C07D 307/79C07C 2601/04
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Claims

Abstract

The present invention is directed to a compound of formula I, and pharmaceutically acceptable salts, solvates, hydrates or stereoisomer thereof, which are useful in treating Syndrome X, Type II diabetes, hyperglycemia, hyperlipidemia, obesity, coagaulopathy, hypertension, arteriosclerosis, and other disorders related to Syndrome X as well as cardiovascular diseases.

Claims

exact text as granted — not AI-modified
1 . A compound of formula I, 
       
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts, solvates, hydrates or stereoisomers thereof, wherein:
 n 1  is 2, 3, 4 or 5; 
 V is a bond or O; 
 X is CH 2  or O; 
 p is 0 or 1; 
 m is 1-4; 
 
       Y 1  is: 
       
         
           
           
               
               
           
         
       
       wherein, 
       
         
           
           
               
               
           
         
       
       is: 1-3-thiazolyl,
 wherein 1-3-thiazolyl are optionally substituted with one or more groups independently selected from the group consisting of: 
 hydrogen, C 1 -C 6  alkyl, C 1 -C 6  alkoxy, halo, haloalkyl and haloalkyloxy; 
 
       Y 1a  is: hydrogen,
 (C 0 -C 3 )alkyl-aryl, 
 C(O)-aryl, 
 heteroaryl, 
 cycloalkyl, 
 heterocycloalkyl, 
 aryloxy, 
 NR 5 (CH 2 ) m OR 5 , 
 aryl-Z-aryl, 
 aryl-Z-heteroaryl, 
 aryl-Z-cycloalkyl, 
 aryl-Z-heterocycloalkyl, 
 heteroaryl-Z-aryl, 
 heteroaryl-Z-heterocycloalkyl or 
 heterocycloalkyl-Z-aryl, 
 wherein aryl, cycloalkyl, aryloxy, heteroaryl, and heterocycloalkyl are optionally substituted with one or more substituents independently selected from the group consisting of:
 halo, 
 hydroxyl, 
 nitro, 
 cyano, 
 C 1 -C 6  alkyl, 
 C 1 -C 6  alkoxy optionally substituted with N(R 5 ) 2 , 
 haloalkyl, 
 N(R 5 ) 2 , 
 N[C(O)R 5 ] 2 , 
 N[S(O) 2 R 5 ] 2 , 
 NR 5 S(O) 2 R 5 , 
 NR 5 C(O)R 5 , 
 NR 5 C(O)OR 5 , 
 C(O)N(R 5 ) 2 , 
 C(O)OR 5  and 
 C(O)R; 
 
 
       Z is: a bond,
 -oxygen- 
 —C(O)NR 5 — 
 —NR 5 C(O)—, 
 —NR 5 C(O)O—, 
 —C(O)—, 
 —NR 5 —, 
 —[O] p (CH 2 ) m —, 
 —(CH 2 ) m [O] p —, 
 —NR 5 (CH 2 ) m — or 
 —(CH 2 ) m  NR 5 —; 
 
       Y 2  and Y 3  are each independently:
 hydrogen, 
 C 1 -C 6  alkyl or 
 C 1 -C 6  alkoxy; 
 
       Y 4  is: (C 1 -C 3 )alkyl-NR 5 C(O)—(C 0 -C 5 )alkyl-Y 7 ,
 (C 1 -C 3 )alkyl-NR 5 C(O)—(C 2 -C 5 )alkenyl-Y 7 , 
 (C 1 -C 3 )alkyl-NR 5 C(O)—(C 2 -C 5 )alkynyl-Y 7 ; 
 (C 1 -C 3 )alkyl-NR 5 C(O)O—(C 0 -C 5 )alkyl-Y 7 , 
 (C 1 -C 3 )alkyl-NR 5 C(O)NR 5 —(C 0 -C 5 )alkyl-Y 7 , 
 (C 1 -C 3 )alkyl-NR 5 C(S)NR 5 —(C 0 -C 5 )alkyl-Y 7 , 
 (C 0 -C 3 )alkyl-C(O)NR 5 —(C 0 -C 5 )alkyl-Y 7 , 
 (C 1 -C 3 )alkyl-OC(O)NY 10 Y 11 , 
 (C 1 -C 3 )alkyl-NY 10 Y 11 , 
 (C 1 -C 3 )alkyl-O—(C 0 -C5)alkyl-Y 7 , 
 (C 1 -C 3 )alkyl-S—(C 0 -C5)alkyl-Y 7  or 
 CN; 
 
       Y 7  is: hydrogen,
 aryl, 
 heteroaryl, 
 C 1 -C 12  alkyl, 
 C 1 -C 6  alkoxy, 
 cycloalkyl, 
 heterocycloalkyl, 
 aryloxy, 
 C(O)-heteroaryl or 
 SR 6 , 
 wherein alkyl, aryl, aryloxy, alkoxy, heteroaryl, cycloalkyl, and heterocycloalkyl are optionally substituted with one or more groups independently selected from R 7 : 
 
       Y 10  and Y 11  are each independently:
 hydrogen, 
 aryl, 
 heteroaryl, 
 C 1 -C 10  alkyl, 
 cycloalkyl, 
 SO 2 (R 6 ); or 
 Y 10  and Y 11  together are a 5- to 10-membered heterocycloalkyl ring or heterocycloalkyl ring fused with aryl, and the heterocycloalkyl ring optionally containing one or more heteroatoms selected from N, O or S; and wherein, aryl, heteroaryl, heterocycloalkyl and alkyl are optionally substituted with one or more substituents independently selected from R 7 ; 
 
       R 5  is: hydrogen or C 1 -C 6  alkyl; 
       R 6  is: hydrogen,
 C 1 -C 10  alkyl, 
 cycloalkyl, 
 aryl, or 
 heteroaryl, 
 wherein alkyl, cycloalkyl, aryl and heteroaryl are optionally substituted with one or more substituents independently selected from R 7 ; 
 
       R 7  is: halo,
 nitro, 
 oxo, 
 cyano, 
 hydroxyl, 
 benzyl, 
 phenyl, 
 phenoxy, 
 heteroaryl, 
 C(O)R 6 , 
 C 1 -C 10  alkyl, 
 C 1 -C 6  alkoxy, 
 C 1 -C 6  haloalkyl, 
 C 1 -C 6  haloalkyloxy, 
 O(CH 2 ) m -phenyl, 
 (CH 2 ) m OC(O)-aryl, 
 C(O)OR 5 , 
 S(O) 2 R 5 , 
 S(O) 2 N(R 5 ) 2 , 
 SR 5  or 
 N(R 5 ) 2 , 
 wherein phenyl and phenoxy are optionally substituted with one or more groups independently selected from halo or trifluoromethyl. 
 
     
     
         2 . The compound of  claim 1 , wherein Y 1a  is selected from the group consisting of: aryl, heteroaryl, cycloalkyl, heterocycloalkyl, aryloxy, 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
     
     
         3 . The compound of  claim 1 , wherein the compound is represented by the following structural formula, 
       
         
           
           
               
               
           
         
       
       wherein E is S. 
     
     
         4 . The compound of  claim 3 , wherein the compound is represented by the following structural formula, 
       
         
           
           
               
               
           
         
       
       wherein q is 1 or 2; and each R 5  is independently hydrogen or methyl. 
     
     
         5 . The compound of  claim 3 , wherein the compound is represented by the following structural formula. 
       
         
           
           
               
               
           
         
       
       wherein q is 1 or 2; and each R 5  is independently hydrogen or methyl. 
     
     
         6 . The compound of  claim 3 , wherein the compound is represented by the following structural formula, 
       
         
           
           
               
               
           
         
       
       wherein q is 1 or 2; and each R 5  is independently hydrogen or methyl. 
     
     
         7 . The compound of  claim 3 , wherein the compound is represented by the following structural formula, 
       
         
           
           
               
               
           
         
       
       wherein q is 0 or 1; and each R 5  is independently hydrogen or methyl. 
     
     
         8 . The compound of  claim 3 , wherein the compound is represented by the following structural formula, 
       
         
           
           
               
               
           
         
       
       wherein q is 1 or 2; and each R 5  is independently hydrogen or methyl. 
     
     
         9 . The compound of  claim 3 , wherein the compound is represented by the following structural formula, 
       
         
           
           
               
               
           
         
       
       wherein q is 1 or 2; and each R 5  is independently hydrogen or methyl. 
     
     
         10 . The compound of  claim 3 , wherein the compound is represented by the following structural formula, 
       
         
           
           
               
               
           
         
       
       wherein q is 1 or 2; and each R 5  is independently hydrogen or methyl. 
     
     
         11 . The compound of  claim 3 , wherein the compound is represented by the following structural Formula, 
       
         
           
           
               
               
           
         
       
       wherein q is 1 or 2; and each R 5 , Y 2  and Y 3  are independently hydrogen or methyl. 
     
     
         12 . (canceled) 
     
     
         13 . (canceled) 
     
     
         14 . The compound of  claim 3 , represented by the following structural formula, 
       
         
           
           
               
               
           
         
       
       wherein Y 1a  is optionally substituted aryl, heteroaryl, heterocycloalkyl, heteroaryl-Z-heterocycloalkyl or heteroaryl-Z-aryl. 
     
     
         15 . (canceled) 
     
     
         16 . (canceled) 
     
     
         17 . The compound of  claim 1  represented by the following structural formula, 
       
         
           
           
               
               
           
         
       
       wherein,
 Y 1a  is hydrogen, aryl, heteroaryl, or aryloxy; q is 1 or 2; and n 1  is 2, 3, or 4. 
 
     
     
         18 . The compound of  claim 1  represented by the following structural formula, 
       
         
           
           
               
               
           
         
       
       wherein,
 Y 1a  is hydrogen, aryl, heteroaryl or aryloxy; q is 1 or 2; and n 1  is 2, 3, or 4. 
 
     
     
         19 . The compound of  claim 1  represented by a following structural formula, 
       
         
           
           
               
               
           
         
       
     
     
         20 . (canceled) 
     
     
         21 . A compound selected from the group consisting of: 
       
         
           
                 
                 
                 
               
                     
                 
                   No. 
                   Compound 
                   Name 
                 
                     
                 
                     
                 
                 
                 
                 
               
                   10 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-{2-(Isopropoxycarbonyl-aminomethyl)-4-[2-(5-methyl-2-morpholin-4-ylthiazol-4-yl)ethoxy]phenyl} propionic acid 
                 
                     
                 
                   20 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-(2-(Isopropoxycarbonyl-aminomethyl)-4-{2-[5-methyl-2-(6-phenylpyridin-3-yl)thiazol-4-yl]ethoxy}phenyl) propionicacid 
                 
                     
                 
                   33 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-(4-{2-[5-Methyl-2-(6-phenylpyridin-3-yl)thiazol-4-yl]ethoxy}-2-{[(pyridine-2-carbonyl)amino]methyl}phenyl)propionic acid HCl salt 
                 
                     
                 
                   43 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-{2-(Cyclopropylmethoxy-carbonylaminomethyl)-4-[2-(5-methyl-2-morpholin-4-ylthiazol-4-yl)ethoxy]phenyl} propionicacid HCl salt 
                 
                     
                 
                   45 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-{2-(Cyclobutoxycarbonyl-aminomethyl)-4-[2-(5-methyl-2-morpholin-4-ylthiazol-4-yl)ethoxy]phenyl} propionic acidHCl salt 
                 
                     
                 
                   54 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-{2-(Isobutoxycarbonyl-aminomethyl)-4-[2-(5-methyl-2-morpholin-4-ylthiazol-4-yl)ethoxy]phenyl} propionic acid 
                 
                     
                 
             
                
                
                
               
               
                
               
            
             
                
                
                
                
                
                
                
                
                
                
                
                
               
            
           
         
       
     
     
         22 . A pharmaceutical composition comprising a pharmaceutically acceptable carrier and a compound of  claim 1  or a pharmaceutically acceptable salt, solvate or hydrate thereof. 
     
     
         23 . (canceled) 
     
     
         24 . A method of modulating a peroxisome proliferator activated receptor (PPAR), comprising the step of contacting the receptor with a compound of  claim 1 , or a pharmaceutically acceptable salt, solvate or hydrate thereof. 
     
     
         25 . (canceled) 
     
     
         26 . (canceled) 
     
     
         27 . (canceled) 
     
     
         28 . A method for lowering blood-glucose comprising the step of administering an effective amount of a compound of  claim 1 . 
     
     
         29 . (canceled) 
     
     
         30 . A method of treating or preventing diabetes mellitus in a mammal comprising the step of administering to a mammal a therapeutically effective amount of a compound of  claim 1 . 
     
     
         31 . A method of treating or preventing cardiovascular disease in a mammal comprising the step of administering to a mammal a therapeutically effective amount of a compound of  claim 1 , or a pharmaceutically acceptable salt, solvate, hydrate or stereoisomer thereof. 
     
     
         32 . A method of treating or preventing syndrome X in a mammal, comprising the step of administering to the mammal a therapeutically effective amount of a compound of  claim 1 , or a pharmaceutically acceptable salt, solvate, hydrate or stereoisomer thereof. 
     
     
         33 . (canceled) 
     
     
         34 . (canceled) 
     
     
         35 . The compound of  claim 5  represented by the following structural formula, 
       
         
           
           
               
               
           
         
       
       or pharmaceutically acceptable salts, solvates, hydrates or stereoisomers thereof. 
     
     
         36 . (canceled)

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