US2005020670A1PendingUtilityA1

Stepwise alkylation of 5-substituted 1-(4-fluorophenyl)-1,3-dihydroisobenzofuran

Assignee: LUNDBECK & CO AS HPriority: Mar 13, 2000Filed: Aug 13, 2004Published: Jan 27, 2005
Est. expiryMar 13, 2020(expired)· nominal 20-yr term from priority
A61P 43/00A61P 9/10A61P 25/28A61P 25/24C07D 307/87C07D 263/52C07D 413/04C07D 277/60C07D 263/10C07D 277/10C07D 417/04A61K 31/343
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Claims

Abstract

Methods for manufacture of citalopram through stepwise alkylation of 5-substituted 1-(4-fluorophenyl)-1,3-dihydroisobenzofurans are disclosed.

Claims

exact text as granted — not AI-modified
1 - 21 . (Canceled)  
     
     
         22 . A compound of the formula V  
       
         
           
           
               
               
           
         
         wherein R represents CN, OH, O-triflate, halogen, NHR 5  wherein R 5  is selected from hydrogen and C 1-6  alkylcarbonyl, CHO, CO 2 R 6 , CONHR 7  wherein R 6 —R 7  are each independently selected from hydrogen and C 1-6  alkyl, or R is a oxazoline or a thiazoline of the formula  
         
           
             
             
                 
                 
             
           
         
         wherein U is O or S;  
         R 1 -R 2  are each independently selected from hydrogen and C 1-6  alkyl, or R 1  and R 2  together form a C 2-5  alkylene chain thereby forming a spiro ring; R 3  is selected from hydrogen and C 1-6  alkyl, R 4  is selected from hydrogen, C 1-6  alkyl, a carboxy group or a precursor group therefor, or R 3  and R 4  together form a C 2-5  alkylene chain thereby forming a spiro ring.  
       
     
     
         23 . A compound according to  claim 22 , wherein R represents CN.  
     
     
         24 . A compound of the formula VI  
       
         
           
           
               
               
           
         
         wherein R represents CN, OH, O-triflate, halogen, NHR 5  wherein R 5  is selected from hydrogen and C 1-6  alkylcarbonyl, CHO, CO 2 R 6 , CONHR 7  wherein R 6 —R 7  are each independently selected from hydrogen and C 1-6  alkyl, or R is a oxazoline or a thiazoline of the formula  
         
           
             
             
                 
                 
             
           
         
         wherein U is O or S;  
         R 1 -R 2  are each independently selected from hydrogen and C 1-6  alkyl, or R 1  and R 2  together form a C 2-5  alkylene chain thereby forming a spiro ring; R 3  is selected from hydrogen and C 1-6  alkyl; R 4  is selected from hydrogen, C 1-6  alkyl, a carboxy group or a precursor group therefor, or R 3  and R 4  together form a C 2-5  alkylene chain thereby forming a spiro ring.  
       
     
     
         25 . A compound of the formula VII  
       
         
           
           
               
               
           
         
         wherein R represents CN, OH, O-triflate, halogen, NHR 5  wherein R 5  is selected from hydrogen and C 1-6  alkylcarbonyl, CHO, CO 2 R 6 , CONHR 7  wherein R 6 -R 7  are each independently selected from hydrogen and C 1-6  alkyl, or R is a oxazoline or a thiazoline of the formula  
         
           
             
             
                 
                 
             
           
         
         wherein U is O or S;  
         R 1 -R 2  are each independently selected from hydrogen and C 1-6  alkyl, or R 1  and R 2  together form a C 2-5  alkylene chain thereby forming a spiro ring; R 3  is selected from hydrogen and C 1-6  alkyl; R 4  is selected from hydrogen, C 1-6  alkyl, a carboxy group or a precursor group therefor, or R 3  and R 4  together form a C 2-5  alkylene chain thereby forming a spiro ring.  
       
     
     
         26 . A compound of the formula VIII  
       
         
           
           
               
               
           
         
         wherein R represents CN, OH, O-triflate, halogen, NHR 5  wherein R 5  is selected from hydrogen and C 1-6  alkylcarbonyl, CHO, CO 2 R 6 , CONHR 7  wherein R 6 -R 7  are each independently selected from hydrogen and C 1-6  alkyl, or R is a oxazoline or a thiazoline of the formula  
         
           
             
             
                 
                 
             
           
         
         wherein U is O or S;  
         R 1 -R 2  are each independently selected from hydrogen and C 1-6  alkyl, or R 1  and R 2  together form a C 2-5  alkylene chain thereby forming a spiro ring; R 3  is selected from hydrogen and C 1-6  alkyl; R 4  is selected from hydrogen, C 1-6  alkyl, a carboxy group or a precursor group therefor, or R 3  and R 4  together form a C 2-5  alkylene chain thereby forming a spiro ring.

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