US2003113622A1PendingUtilityA1

Electrolyte additive for non-aqueous electrochemical cells

Priority: Dec 14, 2001Filed: Dec 14, 2001Published: Jun 19, 2003
Est. expiryDec 14, 2021(expired)· nominal 20-yr term from priority
H01M 4/661H01M 50/145H01M 50/119Y02P70/50H01M 6/166H01M 4/502Y10T29/49108Y02E60/10
46
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Claims

Abstract

An electrochemical secondary cell is disclosed. The cell includes a cathode, an anode, a current collector including aluminum, and an electrolyte containing a perchlorate salt and a second salt. The electrolyte is essentially free of LiPF 6 .

Claims

exact text as granted — not AI-modified
What is claimed is:  
     
         1 . An electrochemical cell comprising a cathode, an anode, a current collector including aluminum, an electrolyte containing a perchlorate salt and a second salt, wherein the electrochemical cell is a secondary cell, and wherein the electrolyte is essentially free of LiPF 6 .  
     
     
         2 . The cell of  claim 1 , wherein the electrolyte contains at least 5000 ppm by weight of a perchlorate salt.  
     
     
         3 . The cell of  claim 2 , wherein the electrolyte contains at least 10,000 ppm by weight of a perchlorate salt.  
     
     
         4 . An electrochemical cell comprising a cathode containing MnO 2 , an anode containing lithium, and an electrolyte containing a perchlorate salt, wherein the cell includes an aluminum surface in electrical contact with a second metal surface, wherein the second metal surface is different than the aluminum surface.  
     
     
         5 . The cell of  claim 4 , wherein the second metal surface is a steel surface.  
     
     
         6 . The cell of  claim 4 , wherein the second metal surface is a stainless steel surface.  
     
     
         7 . The cell of  claim 4 , wherein the second metal surface is an aluminum or aluminum alloy surface.  
     
     
         8 . The cell of  claim 4 , wherein the second metal surface is a nickel surface.  
     
     
         9 . The cell of  claim 4 , wherein the cell includes a cathode current collector comprising aluminum.  
     
     
         10 . The cell of  claim 4 , wherein the electrolyte contains about 500 to about 2500 ppm by weight of the perchlorate salt.  
     
     
         11 . The cell of  claim 4 , wherein the perchlorate salt is LiClO 4 .  
     
     
         12 . The cell of  claim 4 , wherein the perchlorate salt is Ca(ClO 4 ) 2 .  
     
     
         13 . The cell of  claim 4 , wherein the perchlorate salt is Ba(ClO 4 ) 2 .  
     
     
         14 . The cell of  claim 4 , wherein the perchlorate salt is Al(ClO 4 ) 3 .  
     
     
         15 . The cell of  claim 4 , wherein the electrolyte is essentially free of LiPF 6 .  
     
     
         16 . The cell of  claim 4 , wherein the aluminum surface is a portion of an object having at least one dimension greater than 0.5 mm.  
     
     
         17 . The cell of  claim 4 , wherein the aluminum surface is a portion of an object having at least one dimension greater than 1 mm.  
     
     
         18 . The cell of  claim 4 , wherein the aluminum surface is a portion of an object having at least one dimension greater than 2 mm.  
     
     
         19 . An electrochemical cell comprising a cathode containing an aluminum current collector, an anode, and an electrolyte containing a lithium salt and a perchlorate salt, wherein the cell is a primary electrochemical cell.  
     
     
         20 . The cell of  claim 19 , wherein the cathode contains MnO 2 .  
     
     
         21 . The cell of  claim 19 , wherein the anode contains lithium.  
     
     
         22 . The cell of  claim 19 , wherein the electrolyte contains at least 500 ppm by weight of the perchlorate salt.  
     
     
         23 . The cell of  claim 19 , wherein the electrolyte contains at least 1000 ppm by weight of the perchlorate salt.  
     
     
         24 . The cell of  claim 19 , wherein the electrolyte contains at least 1500 ppm by weight of the perchlorate salt.  
     
     
         25 . The cell of  claim 19 , wherein the electrolyte contains at least 2500 ppm by weight of the perchlorate salt.  
     
     
         26 . The cell of  claim 19 , wherein the electrolyte contains less than 20,000 ppm by weight of the perchlorate salt.  
     
     
         27 . The cell of  claim 19 , wherein the perchlorate salt is LiClO 4 .  
     
     
         28 . The cell of  claim 19 , wherein the perchlorate salt is Ca(ClO 4 ) 2 .  
     
     
         29 . The cell of  claim 19 , wherein the perchlorate salt is Ba(ClO 4 ) 2 .  
     
     
         30 . The cell of  claim 19 , wherein the perchlorate salt is Al(ClO 4 ) 3 .  
     
     
         31 . The cell of  claim 19 , wherein the cell includes a case comprising aluminum.  
     
     
         32 . The cell of  claim 31 , wherein the case consists essentially of aluminum.  
     
     
         33 . The cell of  claim 19 , wherein the electrolyte further comprises LiPF 6 .  
     
     
         34 . The cell of  claim 33 , wherein the electrolyte contains at least 5000 ppm by weight LiPF 6 .  
     
     
         35 . The cell of  claim 34 , wherein the electrolyte contains at least 10,000 ppm by weight LiPF 6 .  
     
     
         36 . The cell of  claim 19 , wherein the electrolyte is essentially free of LiPF 6 .  
     
     
         37 . An electrochemical cell comprising a cathode containing MnO 2 , an anode containing lithium, an aluminum surface, and an electrolyte containing about 500 ppm to about 2000 ppm by weight of a perchlorate salt.  
     
     
         38 . The cell of  claim 37 , wherein the perchlorate salt is LiClO 4 .  
     
     
         39 . The cell of  claim 37 , wherein the perchlorate salt is Ca(ClO 4 ) 2 .  
     
     
         40 . The cell of  claim 37 , wherein the perchlorate salt is Ba(ClO 4 ) 2 .  
     
     
         41 . The cell of  claim 37 , wherein the perchlorate salt is Al(ClO 4 ) 3 .  
     
     
         42 . An electrochemical cell comprising a cathode containing MnO 2 , an anode containing lithium, and an electrolyte containing a perchlorate salt, wherein the cell is a primary electrochemical cell, and wherein the cell includes two pieces of aluminum in electrical contact with each other.  
     
     
         43 . A method of inhibiting aluminum corrosion in an electrochemical cell, the method comprising: 
 (a) adding a perchlorate salt to an electrolyte; and    (b) placing the electrolyte, an anode containing Li, and a cathode containing MnO 2  and an aluminum current collector into a cell case to form the cell, wherein the cell is a primary electrochemical cell.    
     
     
         44 . The method of  claim 43 , wherein the perchlorate salt is LiClO 4 .  
     
     
         45 . The method of  claim 43 , wherein the perchlorate salt is Ca(ClO 4 ) 2 .  
     
     
         46 . The method of  claim 43 , wherein the perchlorate salt is Ba(ClO 4 ) 2 .  
     
     
         47 . The method of  claim 43 , wherein the perchlorate salt is Al(ClO 4 ) 3 .

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